Nitrous oxide, known as laughing gas, is the second most-used drug in the UK among 16 to 24-year-olds.

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We show that high-resolution laser spectroscopy can probe surface interactions of gas confined in nanocavities of porous materials. We report on strong line broadening and unfamiliar line shapes due to tight confinement, as well as signal enhancement due to multiple photon scattering. This new domain of laser spectroscopy constitute a challenge for the theory of collisions and spectroscopic line shapes, and open for new ways of analyzing porous materials and processes taking place therein.

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We model the photoelectric emission from and charging of interstellar dust and obtain photoelectric gas heating efficiencies as a function of grain size and the relevant ambient conditions. Using realistic grain size distributions, we evaluate the net gas heating rate for various interstellar environments, and find less heating for dense regions characterized by R_V=5.5 than for diffuse regions with R_V=3.1. We provide fitting functions which reproduce our numerical results for photoelectric heating and recombination cooling for a wide range of interstellar conditions. In a separate paper we will examine the implications of these results for the thermal structure of the interstellar medium. Finally, we investigate the potential importance of photoelectric heating in H II regions, including the warm ionized medium. We find that photoelectric heating could be comparable to or exceed heating due to photoionization of H for high ratios of the radiation intensity to the gas density. We also find that photoelectric heating by dust can account for the observed variation of temperature with distance from the galactic midplane in the warm ionized medium.

We construct an all-sky map of the apparent temperature and optical depth of thermal dust emission using the Planck-HFI and IRAS data. The optical depth maps are correlated to tracers of the atomic and molecular gas. The correlation is linear in the lowest column density regions at high galactic latitudes. At high NH, the correlation is consistent with that of the lowest NH. In the intermediate NH range, we observe departure from linearity, with the dust optical depth in excess to the correlation. We attribute this excess emission to thermal emission by dust associated with a Dark-Gas phase, undetected in the available HI and CO measurements. We show the 2D spatial distribution of the Dark-Gas in the solar neighborhood and show that it extends around known molecular regions traced by CO. The average dust emissivity in the HI phase in the solar neighborhood follows roughly a power law distribution with beta = 1.8 all the way down to 3 mm, although the SED flattens slightly in the millimetre. The threshold for the existence of the Dark-Gas is found at NH = (8.0pm 0.58) 10^{20} Hcm-2. Assuming the same dust emissivity at high frequencies for the dust in the atomic and molecular phases leads to an average XCO = (2.54pm0.13) 10^{20} H2cm-2/(K km s-1). The mass of Dark-Gas is found to be 28% of the atomic gas and 118% of the CO emitting gas in the solar neighborhood. A possible origin for the Dark-Gas is the existence of a dark molecular phase, where H2 survives photodissociation but CO does not. The observed transition for the onset of this phase in the solar neighborhood (AV = 0.4 mag) appears consistent with recent theoretical predictions. We also discuss the possibility that up to half of the Dark-Gas could be in atomic form, due to optical depth effects in the HI measurements.

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Measurements of trace-gases in planetary atmospheres help us explore chemical conditions different to those on Earth. Our nearest neighbor, Venus, has cloud decks that are temperate but hyper-acidic. We report the apparent presence of phosphine (PH3) gas in Venusian atmosphere, where any phosphorus should be in oxidized forms. Single-line millimeter-waveband spectral detections (quality up to ~15 sigma) from the JCMT and ALMA telescopes have no other plausible identification. Atmospheric PH3 at ~20 parts-per-billion abundance is inferred. The presence of phosphine is unexplained after exhaustive study of steady-state chemistry and photochemical pathways, with no currently-known abiotic production routes in Venusian atmosphere, clouds, surface and subsurface, or from lightning, volcanic or meteoritic delivery. Phosphine could originate from unknown photochemistry or geochemistry, or, by analogy with biological production of phosphine on Earth, from the presence of life. Other PH3 spectral features should be sought, while in-situ cloud and surface sampling could examine sources of this gas.